Here's why and some alternatives:
* "Sentiment" is primarily a noun: It refers to a feeling or opinion, often a tender or nostalgic one.
* "To sentiment" is rare: It's considered formal and archaic, mostly used in literary contexts.
* Alternatives are more common: Instead of "to sentiment," consider using verbs like:
* Feel: "She felt a deep sentiment of gratitude."
* Express: "They expressed their sentiments in a letter."
* Hold: "He holds a strong sentiment about family."
* Harbor: "She harbored a sentiment of resentment."
Therefore, while "to sentiment" technically exists, using alternative verbs will be clearer and more widely understood.