If "suitable" means appropriate or fitting:
* Unsuitable
* Inappropriate
* Unfitting
* Inapplicable
If "suitable" means satisfactory or good enough:
* Unsuitable
* Inadequate
* Insufficient
* Unacceptable
If "suitable" means convenient or easy to use:
* Inconvenient
* Awkward
* Difficult
* Unwieldy
The best choice will depend on the specific meaning you want to convey.